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. 2013 May 7;25(17):2404-8.
doi: 10.1002/adma.201204274. Epub 2013 Jan 22.

Two-dimensional supramolecular electron spin arrays

Christian Wäckerlin  1 , Jan Nowakowski, Shi-Xia Liu, Michael Jaggi, Dorota Siewert, Jan Girovsky, Aneliia Shchyrba, Tatjana Hählen, Armin Kleibert, Peter M Oppeneer, Frithjof Nolting, Silvio Decurtins, Thomas A Jung, Nirmalya Ballav
Affiliations

Two-dimensional supramolecular electron spin arrays

Christian Wäckerlin et al. Adv Mater. .

Abstract

A bottom-up approach is introduced to fabricate two-dimensional self-assembled layers of molecular spin-systems containing Mn and Fe ions arranged in a chessboard lattice. We demonstrate that the Mn and Fe spin states can be reversibly operated by their selective response to coordination/decoordination of volatile ligands like ammonia (NH3).

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