Measurements of methane emissions at natural gas production sites in the United States
- PMID: 24043804
- PMCID: PMC3816463
- DOI: 10.1073/pnas.1304880110
Measurements of methane emissions at natural gas production sites in the United States
Erratum in
- Proc Natl Acad Sci U S A. 2013 Oct 29;110(44):18023
Abstract
Engineering estimates of methane emissions from natural gas production have led to varied projections of national emissions. This work reports direct measurements of methane emissions at 190 onshore natural gas sites in the United States (150 production sites, 27 well completion flowbacks, 9 well unloadings, and 4 workovers). For well completion flowbacks, which clear fractured wells of liquid to allow gas production, methane emissions ranged from 0.01 Mg to 17 Mg (mean = 1.7 Mg; 95% confidence bounds of 0.67-3.3 Mg), compared with an average of 81 Mg per event in the 2011 EPA national emission inventory from April 2013. Emission factors for pneumatic pumps and controllers as well as equipment leaks were both comparable to and higher than estimates in the national inventory. Overall, if emission factors from this work for completion flowbacks, equipment leaks, and pneumatic pumps and controllers are assumed to be representative of national populations and are used to estimate national emissions, total annual emissions from these source categories are calculated to be 957 Gg of methane (with sampling and measurement uncertainties estimated at ± 200 Gg). The estimate for comparable source categories in the EPA national inventory is ~1,200 Gg. Additional measurements of unloadings and workovers are needed to produce national emission estimates for these source categories. The 957 Gg in emissions for completion flowbacks, pneumatics, and equipment leaks, coupled with EPA national inventory estimates for other categories, leads to an estimated 2,300 Gg of methane emissions from natural gas production (0.42% of gross gas production).
Keywords: greenhouse gas emissions; hydraulic fracturing.
Conflict of interest statement
Conflict of interest statement: J.M. holds a joint appointment with Barree & Associates and the Colorado School of Mines. She has also served as an advisor to Nexen in 2012. D.T.A. served as a consultant for the Eastern Research Group and ExxonMobil in 2012, and is the current chair of the Science Advisory Board for the EPA. J.H.S. has served as a consultant for Shell in 2012. D.T.A., M.H., C.E.K., and R.F.S. variously serve as members of scientific advisory panels for projects supported by Environmental Defense Fund and companies involved in the natural gas supply chain. These projects are led at Colorado State University (on natural gas gathering and processing), Washington State University (on local distribution of natural gas), and the University of West Virginia (on CNG fueling and use in heavy duty vehicles).
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References
-
- US Environmental Protection Agency (EPA) (2013) Inventory of U.S. Greenhouse Gas Emissions and Sinks: 1990-2011 (Environ Protect Agency, Washington, DC). EPA 430-R-13-001.
-
- Harrison MR, Shires, TM, Wessels JK, Cowgill RM (1996) Methane Emissions from the Natural Gas Industry, Volumes 1–15, Final Report. (Gas Res Inst and Environ Protec Agency, Washington, DC) GRI-94/0257 and EPA-600/R-96-080, Appendix B-1.
-
- Code of Federal Regulations, Title 40 Section 98.233, Calculating GHG Emissions, 75 FR 74488, November 30, 2010, as amended at 76 FR 80575, December 23, 2011.
-
- Energy Information Administration (2013) Annual energy outlook, early release. Available at www.eia.gov/forecasts/aeo/er/index.cfm. Accessed January 31, 2013.
-
- U.S. Environmental Protection Agency (2011) Plan to study the potential impacts of hydraulic fracturing on drinking water resources (Environ Protect Agency, Washington, DC). Available at www2.epa.gov/hfstudy/plan-study-potential-impacts-hydraulic-fracturing-d.... Accessed August 27, 2013.
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