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. 2015 Jan 16;80(2):1235-42.
doi: 10.1021/jo502414w. Epub 2015 Jan 6.

Synthesis of polysubstituted pyrroles via Pd-catalyzed oxidative alkene C-H bond arylation and amination

Jia Zheng  1 , Liangbin Huang, Chuyu Huang, Wanqing Wu, Huanfeng Jiang
Affiliations

Synthesis of polysubstituted pyrroles via Pd-catalyzed oxidative alkene C-H bond arylation and amination

Jia Zheng et al. J Org Chem. .

Abstract

A novel Pd(II)-catalyzed oxidative approach to construct polysubstituted pyrroles from N-homoallylicamines and arylboronic acids was developed. This transformation is supposed to proceed through cascade formation of C-C and C-N bonds via oxidative arylation of unactive alkenes, followed by intramolecular aza-Wacker cyclization.

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