Water at Interfaces

Olle Björneholm¹, Martin H Hansen^{2

3}, Andrew Hodgson⁴, Li-Min Liu^{5

6}, David T Limmer⁷, Angelos Michaelides⁵, Philipp Pedevilla⁵, Jan Rossmeisl³, Huaze Shen⁸, Gabriele Tocci^{5

9}, Eric Tyrode¹⁰, Marie-Madeleine Walz¹, Josephina Werner^{1

11}, Hendrik Bluhm¹²

Affiliations

¹ Department of Physics and Astronomy, Uppsala University , Box 516, 751 20 Uppsala, Sweden.
² Technical University of Denmark , 2800 Kongens Lyngby, Denmark.
³ Department of Chemistry, University of Copenhagen , Universitetsparken 5, 2100 Copenhagen, Denmark.
⁴ Department of Chemistry, University of Liverpool , Liverpool L69 7ZD, United Kingdom.
⁵ Thomas Young Centre, London Centre for Nanotechnology, Department of Physics and Astronomy, and Department of Chemistry, University College London , London WC1E 6BT, United Kingdom.
⁶ Beijing Computational Science Research Center , Beijing, 100193, China.
⁷ Princeton Center for Theoretical Science, Princeton University , Princeton, New Jersey 08544, United States.
⁸ International Center for Quantum Materials and School of Physics, Peking University , Beijing 100871, China.
⁹ Laboratory for fundamental BioPhotonics, Laboratory of Computational Science and Modeling, Institutes of Bioengineering and Materials Science and Engineering, School of Engineering, and Lausanne Centre for Ultrafast Science, École Polytechnique Fédérale de Lausanne (EPFL) , CH-1015 Lausanne, Switzerland.
¹⁰ Department of Chemistry, KTH Royal Institute of Technology , 10044 Stockholm, Sweden.
¹¹ Department of Chemistry and Biotechnology, Swedish University of Agricultural Sciences , Box 7015, 750 07 Uppsala, Sweden.
¹² Chemical Sciences Division, Lawrence Berkeley National Laboratory , Berkeley, California 94720, United States.

PMID: 27232062
DOI: 10.1021/acs.chemrev.6b00045

Free article

Water at Interfaces

Olle Björneholm et al. Chem Rev. 2016.

Free article

. 2016 Jul 13;116(13):7698-726.

doi: 10.1021/acs.chemrev.6b00045. Epub 2016 May 27.

Authors

Affiliations

¹ Department of Physics and Astronomy, Uppsala University , Box 516, 751 20 Uppsala, Sweden.
² Technical University of Denmark , 2800 Kongens Lyngby, Denmark.
³ Department of Chemistry, University of Copenhagen , Universitetsparken 5, 2100 Copenhagen, Denmark.
⁴ Department of Chemistry, University of Liverpool , Liverpool L69 7ZD, United Kingdom.
⁵ Thomas Young Centre, London Centre for Nanotechnology, Department of Physics and Astronomy, and Department of Chemistry, University College London , London WC1E 6BT, United Kingdom.
⁶ Beijing Computational Science Research Center , Beijing, 100193, China.
⁷ Princeton Center for Theoretical Science, Princeton University , Princeton, New Jersey 08544, United States.
⁸ International Center for Quantum Materials and School of Physics, Peking University , Beijing 100871, China.
⁹ Laboratory for fundamental BioPhotonics, Laboratory of Computational Science and Modeling, Institutes of Bioengineering and Materials Science and Engineering, School of Engineering, and Lausanne Centre for Ultrafast Science, École Polytechnique Fédérale de Lausanne (EPFL) , CH-1015 Lausanne, Switzerland.
¹⁰ Department of Chemistry, KTH Royal Institute of Technology , 10044 Stockholm, Sweden.
¹¹ Department of Chemistry and Biotechnology, Swedish University of Agricultural Sciences , Box 7015, 750 07 Uppsala, Sweden.
¹² Chemical Sciences Division, Lawrence Berkeley National Laboratory , Berkeley, California 94720, United States.

PMID: 27232062
DOI: 10.1021/acs.chemrev.6b00045

Abstract

The interfaces of neat water and aqueous solutions play a prominent role in many technological processes and in the environment. Examples of aqueous interfaces are ultrathin water films that cover most hydrophilic surfaces under ambient relative humidities, the liquid/solid interface which drives many electrochemical reactions, and the liquid/vapor interface, which governs the uptake and release of trace gases by the oceans and cloud droplets. In this article we review some of the recent experimental and theoretical advances in our knowledge of the properties of aqueous interfaces and discuss open questions and gaps in our understanding.

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Water at Interfaces

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Water at Interfaces

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