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. 2016 Dec 13;52(100):14478-14481.
doi: 10.1039/c6cc08099e.

Molecular engineering for efficient and selective iron porphyrin catalysts for electrochemical reduction of CO2 to CO

Ram B Ambre  1 , Quentin Daniel  1 , Ting Fan  2 , Hong Chen  1 , Biaobiao Zhang  1 , Lei Wang  1 , Mårten S G Ahlquist  2 , Lele Duan  1 , Licheng Sun  3
Affiliations

Molecular engineering for efficient and selective iron porphyrin catalysts for electrochemical reduction of CO2 to CO

Ram B Ambre et al. Chem Commun (Camb). .

Abstract

Iron porphyrins Fe-pE, Fe-mE, and Fe-oE were synthesized and their electrochemical behavior for CO2 reduction to CO has been investigated. The controlled potential electrolysis of Fe-mE gave exclusive 65% Faradaic efficiency (FE) whereas Fe-oE achieved quasi-quantitative 98% FE (2% H2) for CO production.

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