Measurements of Argon-39 at the U20az underground nuclear explosion site

Abstract

Pacific Northwest National Laboratory reports on the detection of ³⁹Ar at the location of an underground nuclear explosion on the Nevada Nuclear Security Site. The presence of ³⁹Ar was not anticipated at the outset of the experimental campaign but results from this work demonstrated that it is present, along with ³⁷Ar and ⁸⁵Kr in the subsurface at the site of an underground nuclear explosion. Our analysis showed that by using state-of-the-art technology optimized for radioargon measurements, it was difficult to distinguish ³⁹Ar from the fission product ⁸⁵Kr. Proportional counters are currently used for high-sensitivity measurement of ³⁷Ar and ³⁹Ar. Physical and chemical separation processes are used to separate argon from air or soil gas, yielding pure argon with contaminant gases reduced to the parts-per-million level or below. However, even with purification at these levels, the beta decay signature of ⁸⁵Kr can be mistaken for that of ³⁹Ar, and the presence of either isotope increases the measurement background level for the measurement of ³⁷Ar. Measured values for the ³⁹Ar measured at the site ranged from 36,000 milli- Becquerel/standard-cubic-meter-of-air (mBq/SCM) for shallow bore holes to 997,000 mBq/SCM from the rubble chimney from the underground nuclear explosion.

Keywords: Argon-37; Argon-39; Nuclear explosion monitoring; On-site inspection.