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. 2018 Feb 14;140(6):2050-2053.
doi: 10.1021/jacs.7b13220. Epub 2018 Feb 1.

Ni-Catalyzed Site-Selective Dicarboxylation of 1,3-Dienes with CO2

Andreu Tortajada  1 , Ryo Ninokata  1 , Ruben Martin  1   2
Affiliations

Ni-Catalyzed Site-Selective Dicarboxylation of 1,3-Dienes with CO2

Andreu Tortajada et al. J Am Chem Soc. .

Abstract

A site-selective catalytic incorporation of multiple CO2 molecules into 1,3-dienes en route to adipic acids is described. This protocol is characterized by its mild conditions, excellent chemo- and regioselectivity and ease of execution under CO2 (1 atm), including the use of bulk butadiene and/or isoprene feedstocks.

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