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. 2018 Aug 29;47(34):11744-11748.
doi: 10.1039/c8dt02312c.

Octacyanometallate qubit candidates

Tyler J Pearson  1 , Daniel W Laorenza, Matthew D Krzyaniak, Michael R Wasielewski, Danna E Freedman
Affiliations

Octacyanometallate qubit candidates

Tyler J Pearson et al. Dalton Trans. .

Abstract

We report the temperature dependence of the spin dynamics of the octacyanometallates [Mo(CN)8]3- and [W(CN)8]3-. At 5 K, these complexes display remarkably long spin-lattice relaxation times of 1.05 s, and 0.63 s, respectively. We probe the contributing factors to the spin relaxation and demonstrate the impact of spin-orbit coupling as a handle to tune vibrationally mediated spin-lattice relaxation.

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