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. 2018 Sep 13;54(74):10427-10430.
doi: 10.1039/c8cc06334f.

Photochemical and electrochemical hydrogen evolution reactivity of lanthanide-functionalized polyoxotungstates

Marzieh Arab Fashapoyeh  1 , Masoud Mirzaei, Hossein Eshtiagh-Hosseini, Ashwene Rajagopal, Manuel Lechner, Rongji Liu, Carsten Streb
Affiliations

Photochemical and electrochemical hydrogen evolution reactivity of lanthanide-functionalized polyoxotungstates

Marzieh Arab Fashapoyeh et al. Chem Commun (Camb). .

Abstract

The first example of hydrogen evolution reactivity (HER) of lanthanide-functionalized Keggin-based polyoxotungstates under photochemical and electrochemical conditions is reported. The HER activity under homogeneous, visible light-driven conditions and under heterogeneous, electrochemical conditions depends on the type of lanthanide functionalization, so that a new class of model HER catalysts for systematic reactivity studies is now accessible.

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