Response to Comment on "Quantifying hot carrier and thermal contributions in plasmonic photocatalysis"

Linan Zhou¹, Dayne F Swearer², Hossein Robatjazi¹, Alessandro Alabastri¹, Phillip Christopher³, Emily A Carter⁴, Peter Nordlander^{5

6}, Naomi J Halas^{5

2

6}

Affiliations

¹ Department of Electrical and Computer Engineering, Rice University, Houston, TX 77005, USA.
² Department of Chemistry, Rice University, Houston, TX 77005, USA.
³ Department of Chemical Engineering, University of California, Santa Barbara, CA 93106, USA.
⁴ School of Engineering and Applied Science, Princeton University, Princeton, NJ 08544, USA.
⁵ Department of Electrical and Computer Engineering, Rice University, Houston, TX 77005, USA. nordland@rice.edu halas@rice.edu.
⁶ Department of Physics and Astronomy, Rice University, Houston, TX 77005, USA.

PMID: 31048463
DOI: 10.1126/science.aaw9545

Comment

Response to Comment on "Quantifying hot carrier and thermal contributions in plasmonic photocatalysis"

Linan Zhou et al. Science. 2019.

. 2019 May 3;364(6439):eaaw9545.

doi: 10.1126/science.aaw9545. Epub 2019 May 2.

Authors

Linan Zhou¹, Dayne F Swearer², Hossein Robatjazi¹, Alessandro Alabastri¹, Phillip Christopher³, Emily A Carter⁴, Peter Nordlander^{5

6}, Naomi J Halas^{5

2

6}

Affiliations

¹ Department of Electrical and Computer Engineering, Rice University, Houston, TX 77005, USA.
² Department of Chemistry, Rice University, Houston, TX 77005, USA.
³ Department of Chemical Engineering, University of California, Santa Barbara, CA 93106, USA.
⁴ School of Engineering and Applied Science, Princeton University, Princeton, NJ 08544, USA.
⁵ Department of Electrical and Computer Engineering, Rice University, Houston, TX 77005, USA. nordland@rice.edu halas@rice.edu.
⁶ Department of Physics and Astronomy, Rice University, Houston, TX 77005, USA.

PMID: 31048463
DOI: 10.1126/science.aaw9545

Abstract

Sivan et al claim that the methods used to distinguish thermal from hot carrier effects in our recent report are inaccurate and that our data can be explained by a purely thermal mechanism with a fixed activation energy. This conclusion is invalid, because they substantially misinterpret the emissivity of the photocatalyst and assume a linear intensity-dependent temperature in their model that is unrealistic.

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Comment on

Comment on "Quantifying hot carrier and thermal contributions in plasmonic photocatalysis".
Sivan Y, Baraban J, Un IW, Dubi Y. Sivan Y, et al. Science. 2019 May 3;364(6439):eaaw9367. doi: 10.1126/science.aaw9367. Science. 2019. PMID: 31048461

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Response to Comment on "Quantifying hot carrier and thermal contributions in plasmonic photocatalysis"

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Response to Comment on "Quantifying hot carrier and thermal contributions in plasmonic photocatalysis"

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