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. 2019 Jun 26;119(12):6769-6787.
doi: 10.1021/acs.chemrev.9b00045. Epub 2019 May 10.

Recent Advances in Oxidative R1-H/R2-H Cross-Coupling with Hydrogen Evolution via Photo-/Electrochemistry

Huamin Wang  1 , Xinlong Gao  1 , Zongchao Lv  1 , Takfaoui Abdelilah  1 , Aiwen Lei  1   2
Affiliations

Recent Advances in Oxidative R1-H/R2-H Cross-Coupling with Hydrogen Evolution via Photo-/Electrochemistry

Huamin Wang et al. Chem Rev. .

Abstract

Photo-/electrochemical catalyzed oxidative R1-H/R2-H cross-coupling with hydrogen evolution has become an increasingly important issue for molecular synthesis. The dream of construction of C-C/C-X bonds from readily available C-H/X-H with release of H2 can be facilely achieved without external chemical oxidants, providing a greener model for chemical bond formation. Given the great influence of these reactions in organic chemistry, we give a summary of the state of the art in oxidative R1-H/R2-H cross-coupling with hydrogen evolution via photo/electrochemistry, and we hope this review will stimulate the development of a greener synthetic strategy in the near future.

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