Roadmap on halide perovskite and related devices

Abstract

Since the first report on solid-state perovskite solar cells (PSCs) with ∼10% power conversion efficiency (PCE) and 500 h-stability in 2012, tremendous effort has been being devoted to develop PSCs with higher PCE, longer stability and recycling hazardous lead waste. As a result, PCE over 23% was recorded in 2018 and stability over 10 000 h was reported. Beyond photovoltaics, lead halide perovskite materials demonstrated superb properties when they were applied to flat-panel x-ray detectors and non-volatile resistive switching memory. In this review, the progress of the lead halide perovskite in photovoltaics, x-ray imaging and memristors is investigated. Pb-based PSCs and non-Pb-based PSCs are compared, where technologies of non-Pb-based PSCs are not matured for commercialization. Pb-based PSCs were found to be highly suitable for both terrestrial and space photovoltaics. Higher sensitivity under low dose rate observed from the lead halide perovskite suggests a bright future for perovskite x-ray imaging systems. Moreover, high on/off ratio and low energy consumption observed in resistive switching enables perovskite to be a promising candidate for high density memristors.