Large Optical Tunability from Charge Density Waves in 1T-TaS2 under Incoherent Illumination

Abstract

Strongly correlated materials possess a complex energy landscape and host many interesting physical phenomena, including charge density waves (CDWs). CDWs have been observed and extensively studied in many materials since their first discovery in 1972. Yet they present ample opportunities for discovery. Here, we report a large tunability in the optical response of a quasi-2D CDW material, 1T-TaS₂, upon incoherent light illumination at room temperature. We hypothesize that the observed tunability is a consequence of light-induced rearrangement of CDW stacking across the layers of 1T-TaS₂. Our model, based on this hypothesis, agrees reasonably well with experiments suggesting that the interdomain CDW interaction is a vital potentially knob to control the phase of strongly correlated materials.

Keywords: 1T-TaS2; charge density waves; incoherent white light; stacking structure; tunable optical properties.