Vehicle-Deployed Off-Axis Integrated Cavity Output Spectroscopic CH4/C2H6 Sensor System for Mobile Inspection of Natural Gas Leakage

Abstract

A vehicle-deployed parts-per-billion in volume (ppbv)-level off-axis integrated cavity output spectroscopic (OA-ICOS) CH₄/C₂H₆ sensor system was experimentally presented for mobile inspection of natural gas leakage in urban areas. For the time-division-multiplexing-based dual-gas sensor system, an antivibration 35-cm-long optical cavity with an effective path length of ∼2510 m was fabricated with a high-stability temperature and pressure control design. An Allan deviation analysis yielded a minimum detection limit of 0.2 ppbv for CH₄ detection and 10 ppbv for C₂H₆ detection for a 1 s averaging time. A natural gas leakage source location algorithm was proposed using an improved hybrid Nelder-Mead simplex search method and a particle swarm optimization (NM-PSO) algorithm. For field industrial application, the accuracy of the sensor system and leakage source location algorithm was confirmed through a CH₄/C₂H₆ cylinder leakage experiment on the campus. Furthermore, through natural gas pipeline network inspection measurements in urban areas, three types of leakage sources, including natural gas, biogas, and possible leakage source were respectively located and confirmed using the global positioning system and wind speed and direction measurement system, verifying the reliability and potential application of the vehicle-deployed inspection system for future natural gas pipeline leakage monitoring.

Keywords: gas sensor; industrial natural gas; infrared absorption spectroscopy; mobile leakage detection; off-axis integrated cavity output spectroscopy.