Electrostatic precipitator collection efficiency studies using atmospheric radon progeny as aerosol analogs for nuclear explosion radionuclides

Abstract

Electrostatic precipitation (ESP) is an attractive low-powered collection mechanism for mobile and fixed aerosol detection of radionuclides (RNs) for Nuclear Explosion Monitoring (NEM). Aerosol samplers deployed in the International Monitoring System use a blower to draw air through a filter media to collect particulates. ESP-based samplers collect aerosols without a filter, which can greatly increase volumetric flow capacity per watt of power consumed. ESP-based collectors may be optimized to perform low-power mobile RN collection or to improve the air throughput of existing monitoring stations. This effort describes the use of unknown concentrations of atmospheric RNs to determine the collection efficiency of a compact ESP design. For this analysis, naturally occurring radon progeny are simultaneously collected by a single stage wire-plate ESP and a filter-based sampler with a known collection efficiency. The activity of resulting samples is measured with gamma-spectroscopy and decay corrected for analysis time offsets. RN collection efficiencies are then derived for an experimental survey of ESP operational parameters that influence the ionization, transit, and collection of aerosols. At volumetric flow rates of 1.5-2 CMM, the optimized collection efficiency was calculated as 21±2%, and slower rates around 0.5 CMM resulted in 55 ±5% collection efficiency. The monitoring performance of the ESP-based collector was assessed for a simplified nuclear explosion source term by calculating the minimal detectable concentrations of short-lived fission & activation products. Results of the study suggest that a low-power ESP is feasible for NEM at distances of 100s of km.

Keywords: Air sampling; Electrostatic precipitator; Gamma spectroscopy; Nuclear explosion monitoring; Radioactive aerosols; Radon progeny.