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. 2023 Nov 22;23(22):10110-10117.
doi: 10.1021/acs.nanolett.3c02120. Epub 2023 Nov 7.

Multicone Diamond Waveguides for Nanoscale Quantum Sensing

Affiliations

Multicone Diamond Waveguides for Nanoscale Quantum Sensing

Tianqi Zhu et al. Nano Lett. .

Abstract

The long-lived electronic spin of the nitrogen-vacancy (NV) center in diamonds is a promising quantum sensor for detecting nanoscopic magnetic and electric fields in various environments. However, the poor signal-to-noise ratio (SNR) of prevalent optical spin-readout techniques presents a critical challenge in improving measurement sensitivity. Here, we address this limitation by coupling individual NVs to optimized diamond nanopillars, thereby enhancing the collection efficiency of fluorescence. Guided by near-field optical simulations, we predict improved performance for tall (≥5 μm) pillars with tapered sidewalls. This is subsequently verified by fabricating and characterizing a representative set of structures using a newly developed nanofabrication process. We observe increased SNR for optimized devices, owing to improved emission collimation and directionality. Promisingly, these devices are compatible with low-numerical-aperture collection optics and a reduced tip radius, reducing experimental overhead and facilitating improved spatial resolution for scanning applications.

Keywords: diamond nanofabrication; diamond nanophotonics; multicone nanopillar; nitrogen-vacancy center; quantum sensing.

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