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. 2023 Nov 22;23(22):10480-10489.
doi: 10.1021/acs.nanolett.3c03067. Epub 2023 Nov 13.

Shaping Electronic Flows with Strongly Correlated Physics

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Shaping Electronic Flows with Strongly Correlated Physics

Andre Erpenbeck et al. Nano Lett. .

Abstract

Nonequilibrium quantum transport is of central importance in nanotechnology. Its description requires the understanding of strong electronic correlations that couple atomic-scale phenomena to the nanoscale. So far, research in correlated transport has focused predominantly on few-channel transport, precluding the investigation of cross-scale effects. Recent theoretical advances enable the solution of models that capture the interplay between quantum correlations and confinement beyond a few channels. This problem is the focus of this study. We consider an atomic impurity embedded in a metallic nanosheet spanning two leads, showing that transport is significantly altered by tuning only the phase of a single local hopping parameter. Furthermore─depending on this phase─correlations reshape the electronic flow throughout the sheet, either funneling it through the impurity or scattering it away from a much larger region. This demonstrates the potential for quantum correlations to bridge length scales in the design of nanoelectronic devices and sensors.

Keywords: Nanoscale electronics; Nonequilibrium transport; Quantum Monte Carlo; Strongly correlated electron systems.

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