An asymmetric fission island driven by shell effects in light fragments

Abstract

Nuclear fission leads to the splitting of a nucleus into two fragments^1,2. Studying the distribution of the masses and charges of the fragments is essential for establishing the fission mechanisms and refining the theoretical models^3,4. It has value for our understanding of r-process nucleosynthesis^5,6, in which the fission of nuclei with extreme neutron-to-proton ratios is pivotal for determining astrophysical abundances and understanding the origin of the elements⁷ and for energy applications^8,9. Although the asymmetric distribution of fragments is well understood for actinides (elements in the periodic table with atomic numbers from 89 to 103) based on shell effects¹⁰, symmetric fission governs the scission process for lighter elements. However, unexpected asymmetric splits have been observed in neutron-deficient exotic nuclei¹¹, prompting extensive further investigations. Here we present measurements of the charge distributions of fission fragments for 100 exotic fissioning systems, 75 of which have never been measured, and establish a connection between the neutron-deficient sub-lead region and the well-understood actinide region. These new data comprehensively map the asymmetric fission island and provide clear evidence for the role played by the deformed Z = 36 proton shell of the light fragment in the fission of sub-lead nuclei. Our dataset will help constrain the fission models used to estimate the fission properties of nuclei with extreme neutron-to-proton ratios for which experimental data are unavailable.